Atoms irradiated with combined femtosecond laser and extreme ultraviolet (XUV) fields ionize through
multiphoton processes, even when the energy of the XUV photon is below the ionization potential.
However, in the presence of two different XUV photons and an intense laser field, it is possible to induce
full electromagnetic transparency. Taking helium as an example, the laser field modifies its electronic
structure, while the presence of two different XUV photons and the laser field leads to two distinct
ionization pathways that can interfere destructively. This work demonstrates a new approach for coherent
control in a regime of highly excited states and strong optical fields.
http://prl.aps.org/pdf/PRL/v106/i19/e193008
sildes here: http://charles.qols.ph.ic.ac.uk/~twitting/consJCDM/material/20120221_Simon/Journal%20Club%20IC%20Feb21%202012.pptx
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Tuesday, 21 February 2012
Tuesday, 7 February 2012
Richard: Atomic inner-shell X-ray laser at 1.46 nanometres pumped by an X-ray free-electron laser
Atomic inner-shell X-ray laser at 1.46 nanometres pumped by an X-ray free-electron laser
http://www.nature.com/nature/journal/v481/n7382/abs/nature10721.html
Since the invention of the laser more than 50 years ago, scientists have striven to achieve amplification on atomic transitions of increasingly shorter wavelength1, 2, 3, 4, 5, 6, 7. The introduction of X-ray free-electron lasers8, 9, 10makes it possible to pump new atomic X-ray lasers11, 12, 13 with ultrashort pulse duration, extreme spectral brightness and full temporal coherence. Here we describe the implementation of an X-ray laser in the kiloelectronvolt energy regime, based on atomic population inversion and driven by rapid K-shell photo-ionization using pulses from an X-ray free-electron laser. We established a population inversion of the Kα transition in singly ionized neon14at 1.46 nanometres (corresponding to a photon energy of 849 electronvolts) in an elongated plasma column created by irradiation of a gas medium. We observed strong amplified spontaneous emission from the end of the excited plasma. This resulted in femtosecond-duration, high-intensity X-ray pulses of much shorter wavelength and greater brilliance than achieved with previous atomic X-ray lasers. Moreover, this scheme provides greatly increased wavelength stability, monochromaticity and improved temporal coherence by comparison with present-day X-ray free-electron lasers. The atomic X-ray lasers realized here may be useful for high-resolution spectroscopy and nonlinear X-ray studies.
http://www.nature.com/nature/journal/v481/n7382/abs/nature10721.html
Since the invention of the laser more than 50 years ago, scientists have striven to achieve amplification on atomic transitions of increasingly shorter wavelength1, 2, 3, 4, 5, 6, 7. The introduction of X-ray free-electron lasers8, 9, 10makes it possible to pump new atomic X-ray lasers11, 12, 13 with ultrashort pulse duration, extreme spectral brightness and full temporal coherence. Here we describe the implementation of an X-ray laser in the kiloelectronvolt energy regime, based on atomic population inversion and driven by rapid K-shell photo-ionization using pulses from an X-ray free-electron laser. We established a population inversion of the Kα transition in singly ionized neon14at 1.46 nanometres (corresponding to a photon energy of 849 electronvolts) in an elongated plasma column created by irradiation of a gas medium. We observed strong amplified spontaneous emission from the end of the excited plasma. This resulted in femtosecond-duration, high-intensity X-ray pulses of much shorter wavelength and greater brilliance than achieved with previous atomic X-ray lasers. Moreover, this scheme provides greatly increased wavelength stability, monochromaticity and improved temporal coherence by comparison with present-day X-ray free-electron lasers. The atomic X-ray lasers realized here may be useful for high-resolution spectroscopy and nonlinear X-ray studies.
Additional Info:
Jon's News&Views: http://www.nature.com/nature/journal/v481/n7382/full/481452a.html
Tuesday, 31 January 2012
Seb: Hollow core fiber at 1.8microns
Trallero-Herrero,
C., Jin, C., Schmidt, B. E., Shiner, a D., Kieffer, J.-C., Corkum,
P. B., Villeneuve, D. M., et al. (2012). Generation of broad XUV
continuous high harmonic spectra and isolated attosecond pulses
with intense mid-infrared lasers. Journal of Physics B:
Atomic, Molecular and Optical Physics, 45(1),
011001. doi:10.1088/0953-4075/45/1/ 011001
Shiner, a. D.,
Schmidt, B. E., Trallero-Herrero, C., Wörner, H. J., Patchkovskii,
S., Corkum, P. B., Kieffer, J.-C., et al. (2011). Probing
collective multi-electron dynamics in xenon with high-harmonic
spectroscopy. Nature Physics, 7(6), 464-467.
Nature Publishing Group. doi:10.1038/nphys1940
paper: http://www.nature.com/nphys/journal/v7/n6/full/nphys1940.html
supplementary information (a lot of material): http://www.nature.com/nphys/journal/v7/n6/extref/nphys1940-s1.pdf
Tuesday, 24 January 2012
Tuesday, 17 January 2012
JC: Felix: Optimal pulse compression in long hollow fibers
Optimal pulse compression in long hollow fibers
by Nagy, Tamas, Vladimir Pervak, and Peter Simon
Tuesday, 10 January 2012
DM: Simon: XUV Initiated High Harmonic Generation
I intend on giving a thorough and descriptive introduction so if you'd
like to learn more about what I'm trying to do in my project - this
would be a good opportunity to find out! Also, if you think that your
wisdom might add to the discussion, please come
along - as I would value external insight.
Wednesday, 14 December 2011
DM: Suren: Attosecond cascades and time-delays in one-electron photo-ionization
I shall present time-resolved ab-initio study of the attosecond dynamics
of electron-electron correlation during single-electron, single
XUV-photon ionization of an excited two-electron atom. Specifically, we
aim to time-resolve the two fundamental processes that play the key role
in electronic excitations of the ion created by ionization: the
shake-up and the post-ionization interaction of the outgoing electron
with the core (knock-up). These two processes have different time
characteristics: while the shake-up is an essentially instantaneous
process, the knock-up excitation due to the interaction between the
ionic and the continuum electrons depends on the movement of the latter
and may be significant for longer times, leading to delays in the
ionization process. We observe an interplay of the initial shake-up
excitation with the excitation cascades induced by the post-ionization
interaction of the outgoing electron with the core. The time-scales and
the structure of these excitation cascades is directly linked to the
time it takes the 'active' continuum electron, lifted from a deeper
bound orbital, to traverse the orbit of the 'passive' electron residing
in the outer orbit. Ideas for resolving and controlling the two-electron
interaction dynamics during the ionization process will be discussed.
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