They carry out HHG in Methane and Xeon using two colours and show a
suppression of the HHG signal in Methane in the presence of a .weak.
1500-1900 field from an OPA which is resonant with a vibration
transition in Methane. This has quite a lot of cross over with work
that has been done or is being carried out with the Red Dragon lab.
We experimentally investigate the high harmonic generation (HHG) from
CH4 molecules and Xe atoms in a two-color field (using the 800nm laser
and the tunable laser with the longer wavelength from 1500nm to 1900nm),
and observe that the longer wavelength component can destructively
suppress the HHG from CH4 molecules. By controlling the time delay
between the two color laser pulses or tuning the laser intensity of the
longer wavelength component, the suppressions of the HHG from CH4
molecules and the enhancements of the HHG from Xe atoms at the same
laser condition are observed. The results indicate that the longer
wavelength component around the molecular infrared absorption can
suppress the molecular HHG process.
http://www.opticsinfobase.org/abstract.cfm?uri=oe-18-11-11664
PPT slides to follow...
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Tuesday, 23 November 2010
Tuesday, 16 November 2010
JC: Will: Higher-Order Kerr Terms Allow Ionization-Free Filamentation in Gases
We show that higher-order nonlinear indices (n4, n6, n8, n10) provide
the main defocusing contribution to self-channeling of ultrashort laser
pulses in air and argon at 800 nm, in contrast with the previously
accepted mechanism of filamentation where plasma was considered as the
dominant defocusing process. Their consideration allows us to reproduce
experimentally observed intensities and plasma densities in self-guided
filaments.
http://prl.aps.org/abstract/PRL/v104/i10/e103903
PPT slides and other material here
http://prl.aps.org/abstract/PRL/v104/i10/e103903
PPT slides and other material here
Tuesday, 9 November 2010
DM: Rashid: High-order Harmonic Generation of Laser Radiation in Plasmas: Recent Achievements and Perspectives
Resent research on high-order harmonic generation in laser-produced
plasmas is reviewed. We analyze the conditions for the generation of
harmonics (up to the 101st order, . ~ 7.9 nm) in the propagation of
laser radiation through a weakly-ionized plasma prepared by irradiating
the surfaces of different targets with a laser prepulse. First
experiments on attosecond pulse generation from plasma plumes are
presented. We discuss the findings of investigations into the resonance
intensity enhancement of individual harmonics in a number of plasma
formations, which have demonstrated a substantial increase in the
conversion efficiency in the plateau region of the harmonic distribution
(in particular, of the 13th harmonic in indium plasmas with the
efficiency 10-4). We review the results of investigations of harmonic
generation in nanoparticle-containing plasmas (metallic clusters,
fullerenes, nanotubes). Different techniques for increasing the
intensity and order of the generated harmonics are discussed. Future
perspectives are analyzed as well. Among them are: (a) high-power
harmonics from nanoclusters at 1 kHz pulse repetition rates, (b)
few-cycle pump-induced harmonics, (c) molecular orientation in plasma
plumes, (d) attosecond experiments, (e) plasma manipulations, (e)
carbon-containing plasma: perspectives of application for plasma HHG,
(f) long-wavelength femtosecond pump.
PPT slides and other material here
PPT slides and other material here
Tuesday, 2 November 2010
DM: Amelle: Molecular QPI
I will discuss our recent result on molecular internal dynamics studied
by quantum path interferences in high order harmonic. Upon a certain
number a available technique we are looking in providing one that is
self-referenced and will allowed to access information on the nuclear
and electron dynamics of the cation created in the time scale of the HHG
process.
Tuesday, 26 October 2010
JC: Sebastien: Mapping Molecular Orbital Symmetriy on High-Order Harmonic Generation Spectrum Using Two-Color Laser Fields
We have measured high-order harmonic generation spectra of D2, N2, and
CO2 by mixing orthogonally polarized 800 and 400 nm laser fields. The
intensity of the high-harmonic spectrum is modulated as we change the
relative phase of the two pulses. For randomly orientated molecules, the
phase of the intensity modulation depends on the symmetry of the
molecular orbitals from which the high harmonics are emitted. This
allows us to identify the symmetry of any orbital that contributes to
high-harmonic generation, even without aligning the molecule. Our
approach can be a route to imaging dynamical changes in
three-dimensional molecular orbitals on a time scale as short as a few
hundred attoseconds.
http://prl.aps.org/abstract/PRL/v105/i5/e053003
http://prl.aps.org/abstract/PRL/v105/i5/e053003
Tuesday, 19 October 2010
DM: Chris Arrell: Thesis and Surface Science Experiments Outlook
I will present measurements from the surface science apparatus and
discuss the next steps for the project. Measurements have shown
evidence of localised plasmonic enhancement from silver and
'hot-electron' temporal dynamics on an Au surface
Tuesday, 12 October 2010
JC: Richard: Inconsistencies between two attosecond pulse metrology methods: A comparative study
The two basic approaches underlying most of the metrology of attosecond
pulse trains are compared in the spectral region ~14-24 eV, that is,
the second-order intensity volume autocorrelation and the resolution of
attosecond beating by interference of two photon transitions (RABITT).
They give rather dissimilar pulse durations. It is concluded that for
the present experimental conditions RABITT may underestimate the
duration under measurement, due to variations of the driving intensity,
but in conjunction with theory allows an estimation of the relative
contributions of two different electron trajectories to the
extreme-ultraviolet (XUV) radiation.
http://pra.aps.org/abstract/PRA/v82/i2/e021402
PPT slides...
http://pra.aps.org/abstract/PRA/v82/i2/e021402
PPT slides...
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